44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 03 12 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 34697.25 -2.7 999999.9 999999.9 34732.25 2.9 999999.9 999999.9 34767.25 11.1 999999.9 999999.9 34802.25 5.5 999999.9 999999.9 34837.25 -17.6 999999.9 999999.9 34872.25 12.1 999999.9 999999.9 34907.25 9.0 999999.9 999999.9 34942.25 16.1 999999.9 999999.9 34977.25 27.2 999999.9 999999.9 35012.25 12.7 999999.9 999999.9 35047.25 5.8 999999.9 999999.9 35082.25 999999.9 999999.9 999999.9 35117.25 28.8 999999.9 999999.9 35152.25 46.7 999999.9 999999.9 35187.25 39.6 999999.9 999999.9 35222.25 34.1 999999.9 999999.9 35257.25 28.3 999999.9 999999.9 35292.25 43.4 999999.9 999999.9 35327.25 132.3 999999.9 999999.9 35362.25 68.0 999999.9 999999.9 35397.25 999999.9 999999.9 999999.9 35432.25 91.9 999999.9 999999.9 35467.25 124.2 999999.9 999999.9 35502.25 139.9 999999.9 999999.9 35537.25 117.0 999999.9 999999.9 35572.25 144.1 999999.9 999999.9 35607.25 142.2 999999.9 999999.9 35642.25 235.7 999999.9 999999.9 35677.25 167.3 999999.9 999999.9 35712.25 228.3 999999.9 475.3 35747.25 313.4 999999.9 999999.9 35782.25 275.3 76.3 999999.9 35817.25 368.5 82.6 999999.9 35852.25 416.8 999999.9 999999.9 35887.25 451.4 999999.9 999999.9 35922.25 367.1 999999.9 999999.9 35957.25 381.9 999999.9 999999.9 35992.25 441.2 113.3 999999.9 36027.25 547.2 119.7 999999.9 36062.25 508.8 102.2 999999.9 36097.25 544.1 999999.9 564.1 36132.25 572.0 999999.9 999999.9 36167.25 577.3 999999.9 999999.9 36202.25 560.5 100.5 999999.9 36237.25 664.4 99.3 999999.9 36272.25 762.1 999999.9 999999.9 36307.25 728.7 999999.9 999999.9 36342.25 753.9 999999.9 999999.9 36377.25 756.0 999999.9 999999.9 36412.25 871.5 999999.9 999999.9 36447.25 869.8 999999.9 999999.9 36482.25 810.6 999999.9 999999.9 36517.25 813.4 999999.9 999999.9 36552.25 785.7 999999.9 999999.9 36587.25 809.6 999999.9 999999.9 36622.25 780.3 999999.9 999999.9 36657.25 832.3 174.7 999999.9 36692.25 867.0 184.3 999999.9 36727.25 803.5 177.4 999999.9 36762.25 875.6 999999.9 359.1 36797.25 855.2 999999.9 417.1 36832.25 835.6 999999.9 999999.9 36867.25 896.3 161.7 999999.9 36902.25 875.0 167.6 999999.9 36937.25 915.2 999999.9 999999.9 36972.25 858.7 999999.9 999999.9 37007.25 818.4 999999.9 999999.9 37042.25 891.7 999999.9 999999.9 37077.25 883.7 151.6 999999.9 37112.25 950.7 185.9 999999.9 37147.25 894.0 172.2 999999.9 37182.25 888.9 999999.9 343.0 37217.25 832.8 999999.9 999999.9 37252.25 895.6 999999.9 999999.9 37287.25 870.4 132.1 999999.9 37322.25 828.5 140.9 999999.9 37357.25 845.2 999999.9 999999.9 37392.25 821.2 999999.9 999999.9 37427.25 787.6 999999.9 999999.9 37462.25 856.2 999999.9 999999.9 37497.25 822.3 140.8 999999.9 37532.25 922.3 142.5 999999.9 37567.25 816.3 125.7 999999.9 37602.25 851.2 999999.9 611.8 37637.25 842.1 999999.9 632.4 37672.25 815.0 999999.9 999999.9 37707.25 818.3 999999.9 999999.9 37742.25 791.0 105.9 999999.9 37777.25 811.0 999999.9 999999.9 37812.25 821.5 999999.9 999999.9 37847.25 842.8 999999.9 999999.9 37882.25 826.6 999999.9 999999.9 37917.25 915.0 999999.9 999999.9 37952.25 959.6 999999.9 999999.9 37987.25 1002.8 999999.9 999999.9 38022.25 1004.1 999999.9 999999.9 38057.25 945.6 999999.9 999999.9 38092.25 927.1 999999.9 999999.9 38127.25 886.3 999999.9 999999.9 38162.25 870.2 160.2 999999.9 38197.25 845.4 142.3 999999.9 38232.25 913.8 123.7 999999.9 38267.25 878.3 999999.9 621.2 38302.25 858.6 999999.9 675.0 38337.25 867.7 999999.9 999999.9 38372.25 840.5 999999.9 999999.9 38407.25 924.4 131.1 999999.9 38442.25 913.7 999999.9 999999.9 38477.25 901.5 999999.9 999999.9 38512.25 931.2 999999.9 999999.9 38547.25 867.8 999999.9 999999.9 38582.25 837.5 157.7 999999.9 38617.25 875.6 131.9 999999.9 38652.25 901.3 145.1 999999.9 38687.25 842.3 999999.9 578.2 38722.25 849.2 999999.9 999999.9 38757.25 857.0 999999.9 999999.9 38792.25 907.7 999999.9 999999.9 38827.25 843.3 123.7 999999.9 38862.25 893.2 999999.9 999999.9 38897.25 932.8 999999.9 999999.9 38932.25 925.6 999999.9 999999.9 38967.25 857.0 999999.9 999999.9 39002.25 863.5 144.6 999999.9 39037.25 865.7 123.6 999999.9 39072.25 860.4 140.7 999999.9 39107.25 832.8 999999.9 667.3 39142.25 868.6 999999.9 626.2 39177.25 872.3 999999.9 999999.9 39212.25 862.8 999999.9 999999.9 39247.25 824.5 131.8 999999.9 39282.25 890.5 999999.9 999999.9 39317.25 874.1 999999.9 999999.9 39352.25 890.9 999999.9 999999.9 39387.25 953.4 999999.9 999999.9 39422.25 1002.8 999999.9 999999.9 39457.25 1001.3 999999.9 999999.9 39492.25 971.7 999999.9 999999.9 39527.25 1040.7 999999.9 999999.9 39562.25 900.8 999999.9 999999.9 39597.25 877.5 999999.9 999999.9 39632.25 923.3 999999.9 999999.9 39667.25 948.2 169.7 999999.9 39702.25 946.9 170.7 999999.9 39737.25 958.8 157.9 999999.9 39772.25 897.4 999999.9 362.6 39807.25 939.6 999999.9 442.1 39842.25 910.7 999999.9 999999.9 39877.25 933.8 130.9 999999.9 39912.25 961.3 135.4 999999.9 39947.25 961.9 999999.9 999999.9 39982.25 989.2 999999.9 999999.9 40017.25 921.8 999999.9 999999.9 40052.25 919.8 999999.9 999999.9 40087.25 906.8 149.2 999999.9 40122.25 843.8 145.9 999999.9 40157.25 908.2 116.4 999999.9 40192.25 842.3 999999.9 679.3 40227.25 826.6 999999.9 665.9 40262.25 872.9 999999.9 999999.9 40297.25 912.7 999999.9 999999.9 40332.25 877.8 127.1 999999.9 40367.25 1022.1 999999.9 999999.9 40402.25 1035.4 999999.9 999999.9 40437.25 1027.1 999999.9 999999.9 40472.25 1012.7 999999.9 999999.9 40507.25 1018.7 192.3 999999.9 40542.25 1083.4 194.4 999999.9 40577.25 1036.6 199.1 999999.9 40612.25 1048.6 999999.9 274.9 40647.25 1010.0 999999.9 999999.9 40682.25 1013.9 999999.9 999999.9 40717.25 984.1 999999.9 999999.9 40752.25 1009.5 179.6 999999.9 40787.25 1067.4 999999.9 999999.9 40822.25 1025.7 999999.9 999999.9 40857.25 998.1 999999.9 999999.9 40892.25 1047.4 999999.9 999999.9 40927.25 1093.1 999999.9 999999.9 40962.25 1127.1 999999.9 999999.9 40997.25 1062.0 999999.9 999999.9 41032.25 1039.4 999999.9 999999.9 41067.25 1049.4 999999.9 999999.9 41102.25 1035.0 999999.9 999999.9 41137.25 998.1 999999.9 999999.9 41172.25 973.1 190.1 999999.9 41207.25 953.7 178.7 999999.9 41242.25 955.4 194.5 999999.9 41277.25 943.6 999999.9 285.8 41312.25 986.7 999999.9 284.2 41347.25 942.5 999999.9 999999.9 41382.25 1014.1 999999.9 999999.9 41417.25 952.9 167.0 999999.9 41452.25 976.6 999999.9 999999.9 41487.25 958.8 999999.9 999999.9 41522.25 944.2 999999.9 999999.9 41557.25 1028.7 999999.9 999999.9 41592.25 949.1 192.0 999999.9 41627.25 944.3 181.3 999999.9 41662.25 943.6 196.2 999999.9 41697.25 947.9 999999.9 307.9 41732.25 930.4 999999.9 372.7 41767.25 900.8 999999.9 999999.9 41802.25 930.7 999999.9 999999.9 41837.25 974.0 183.0 999999.9 41872.25 978.7 999999.9 999999.9 41907.25 970.9 999999.9 999999.9 41942.25 998.7 999999.9 999999.9 41977.25 978.0 999999.9 999999.9 42012.25 969.5 209.6 999999.9 42047.25 957.9 189.8 999999.9 42082.25 932.5 174.6 999999.9 42117.25 923.0 999999.9 416.4 42152.25 933.0 999999.9 999999.9 42187.25 913.7 999999.9 999999.9 42222.25 950.9 999999.9 999999.9 42257.25 891.7 159.3 999999.9 42292.25 953.8 999999.9 999999.9 42327.25 940.5 999999.9 999999.9 42362.25 939.8 999999.9 999999.9 42397.25 949.6 999999.9 999999.9 42432.25 956.7 999999.9 999999.9 42467.25 951.7 999999.9 999999.9 42502.25 982.4 999999.9 999999.9 42537.25 974.2 999999.9 999999.9 42572.25 991.4 999999.9 999999.9 42607.25 986.6 999999.9 999999.9 42642.25 919.7 999999.9 999999.9 42677.25 935.0 208.6 999999.9 42712.25 922.0 178.7 999999.9 42747.25 932.0 190.3 999999.9 42782.25 891.3 999999.9 419.6 42817.25 883.7 999999.9 464.0 42852.25 857.1 999999.9 999999.9 42887.25 880.8 150.3 999999.9 42922.25 850.7 159.1 999999.9 42957.25 952.1 999999.9 999999.9 42992.25 870.7 999999.9 999999.9 43027.25 936.5 999999.9 999999.9 43062.25 887.2 999999.9 999999.9 43097.25 912.8 171.2 999999.9 43132.25 889.4 176.0 999999.9 43167.25 921.8 163.9 999999.9 43202.25 894.3 999999.9 447.4 43237.25 938.5 999999.9 468.3 43272.25 946.0 999999.9 999999.9 43307.25 953.8 154.9 999999.9 43342.25 926.7 164.3 999999.9 43377.25 929.0 999999.9 999999.9 43412.25 918.2 999999.9 999999.9 43447.25 912.9 999999.9 999999.9 43482.25 937.0 999999.9 999999.9 43517.25 925.3 182.5 999999.9 43552.25 883.1 174.1 999999.9 43587.25 944.7 184.2 999999.9 43622.25 885.3 999999.9 424.8 43657.25 866.5 999999.9 398.4 43692.25 882.6 999999.9 999999.9 43727.25 860.7 171.6 999999.9 43762.25 936.7 160.4 999999.9 43797.25 919.9 999999.9 999999.9 43832.25 931.9 999999.9 999999.9 43867.25 927.0 999999.9 999999.9 43902.25 955.1 999999.9 999999.9 43937.25 1000.4 999999.9 999999.9 43972.25 957.5 999999.9 999999.9 44007.25 963.6 999999.9 999999.9 44042.25 976.4 999999.9 999999.9 44077.25 892.8 999999.9 999999.9 44112.25 933.4 999999.9 999999.9 44147.25 935.1 999999.9 999999.9 44182.25 907.3 214.1 999999.9 44217.25 988.7 199.8 999999.9 44252.25 913.3 206.4 999999.9 44287.25 972.5 999999.9 266.0 44322.25 942.8 999999.9 302.8 44357.25 942.8 999999.9 999999.9 44392.25 897.6 999999.9 999999.9 44427.25 900.9 196.4 999999.9 44462.25 963.9 999999.9 999999.9 44497.25 962.6 999999.9 999999.9 44532.25 964.2 999999.9 999999.9 44567.25 913.9 999999.9 999999.9 44602.25 892.2 216.4 999999.9 44637.25 898.5 198.6 999999.9 44672.25 851.4 162.9 999999.9 44707.25 838.2 999999.9 568.2 44742.25 839.6 999999.9 590.4 44777.25 844.2 999999.9 999999.9 44812.25 847.5 999999.9 999999.9 44847.25 859.2 157.0 999999.9 44882.25 872.9 999999.9 999999.9 44917.25 805.2 999999.9 999999.9 44952.25 823.2 999999.9 999999.9 44987.25 855.5 999999.9 999999.9 45022.25 757.5 186.0 999999.9 45057.25 780.1 167.8 999999.9 45092.25 744.8 147.0 999999.9 45127.25 738.8 999999.9 734.4 45162.25 722.2 999999.9 999999.9 45197.25 701.5 999999.9 999999.9 45232.25 746.2 999999.9 999999.9 45267.25 753.8 158.2 999999.9 45302.25 827.4 999999.9 999999.9 45337.25 767.5 999999.9 999999.9 45372.25 765.0 999999.9 999999.9 45407.25 821.2 999999.9 999999.9 45442.25 853.8 999999.9 999999.9 45477.25 800.5 999999.9 999999.9 45512.25 819.6 999999.9 999999.9 45547.25 868.3 999999.9 999999.9 45582.25 854.1 999999.9 999999.9 45617.25 830.7 999999.9 999999.9 45652.25 800.6 999999.9 999999.9 45687.25 850.4 200.1 999999.9 45722.25 789.0 153.4 999999.9 45757.25 832.5 156.1 999999.9 45792.25 771.0 999999.9 690.9 45827.25 834.4 999999.9 618.1 45862.25 853.4 999999.9 999999.9 45897.25 895.8 999999.9 999999.9 45932.25 884.7 200.4 999999.9 45967.25 891.4 999999.9 999999.9 46002.25 814.6 999999.9 999999.9 46037.25 920.3 999999.9 999999.9 46072.25 915.0 999999.9 999999.9 46107.25 852.2 224.2 999999.9 46142.25 838.5 211.2 999999.9 46177.25 957.1 209.8 999999.9 46212.25 946.8 999999.9 405.2 46247.25 928.7 999999.9 999999.9 46282.25 896.3 999999.9 999999.9 46317.25 917.8 999999.9 999999.9 46352.25 859.4 232.3 999999.9 46387.25 945.4 999999.9 999999.9 46422.25 855.9 999999.9 999999.9 46457.25 870.2 999999.9 999999.9 46492.25 852.4 999999.9 999999.9 46527.25 864.8 225.0 999999.9 46562.25 839.9 242.2 999999.9 46597.25 883.6 252.6 999999.9 46632.25 852.7 999999.9 352.1 46667.25 823.5 999999.9 999999.9 46702.25 809.5 999999.9 999999.9 46737.25 850.8 247.3 999999.9 46772.25 912.4 246.1 999999.9 46807.25 894.6 999999.9 999999.9 46842.25 908.9 999999.9 999999.9 46877.25 928.7 999999.9 999999.9 46912.25 915.5 999999.9 999999.9 46947.25 933.7 999999.9 999999.9 46982.25 894.4 999999.9 999999.9 47017.25 922.1 999999.9 999999.9 47052.25 917.4 999999.9 999999.9 47087.25 810.2 999999.9 999999.9 47122.25 847.3 999999.9 999999.9 47157.25 805.2 999999.9 999999.9 47192.25 870.0 268.6 999999.9 47227.25 797.9 251.1 999999.9 47262.25 794.3 265.2 999999.9 47297.25 768.8 999999.9 406.4 47332.25 813.0 999999.9 376.9 47367.25 739.6 999999.9 999999.9 47402.25 763.0 999999.9 999999.9 47437.25 773.2 239.7 999999.9 47472.25 814.4 999999.9 999999.9 47507.25 826.3 999999.9 999999.9 47542.25 746.6 999999.9 999999.9 47577.25 789.5 999999.9 999999.9 47612.25 772.4 264.5 999999.9 47647.25 712.0 237.9 999999.9 47682.25 777.8 241.4 999999.9 47717.25 787.5 999999.9 493.2 47752.25 720.4 999999.9 524.1 47787.25 727.8 999999.9 999999.9 47822.25 779.3 999999.9 999999.9 47857.25 739.0 246.5 999999.9 47892.25 823.1 999999.9 999999.9 47927.25 770.3 999999.9 999999.9 47962.25 746.6 999999.9 999999.9 47997.25 772.0 999999.9 999999.9 48032.25 746.9 283.8 999999.9 48067.25 731.9 260.4 999999.9 48102.25 737.3 265.7 999999.9 48137.25 705.1 999999.9 452.4 48172.25 730.8 999999.9 504.6 48207.25 731.1 999999.9 999999.9 48242.25 730.0 999999.9 999999.9 48277.25 724.6 286.1 999999.9 48312.25 743.7 999999.9 999999.9 48347.25 689.3 999999.9 999999.9 48382.25 713.3 999999.9 999999.9 48417.25 716.2 999999.9 999999.9 48452.25 680.9 999999.9 999999.9 48487.25 724.4 999999.9 999999.9 48522.25 706.1 999999.9 999999.9 48557.25 729.8 999999.9 999999.9 48592.25 649.0 999999.9 999999.9 48627.25 668.3 999999.9 999999.9 48662.25 690.8 999999.9 999999.9 48697.25 671.9 337.0 999999.9 48732.25 643.4 330.3 999999.9 48767.25 666.3 319.8 999999.9 48802.25 554.6 999999.9 417.6 48837.25 558.4 999999.9 415.7 48872.25 540.2 999999.9 999999.9 48907.25 539.2 999999.9 999999.9 48942.25 509.3 268.1 999999.9 48977.25 577.9 999999.9 999999.9 49012.25 525.3 999999.9 999999.9 49047.25 367.7 999999.9 999999.9 49082.25 385.5 999999.9 999999.9 49117.25 399.9 263.5 999999.9 49152.25 319.7 191.1 999999.9 49187.25 304.1 181.7 999999.9 49222.25 187.2 999999.9 709.6 49257.25 161.7 999999.9 999999.9 49292.25 142.6 999999.9 999999.9 49327.25 157.6 53.9 999999.9 49362.25 135.2 66.2 999999.9 49397.25 115.7 999999.9 999999.9 49432.25 73.9 999999.9 999999.9 49467.25 94.9 999999.9 999999.9 49502.25 89.7 999999.9 999999.9 49537.25 121.1 73.3 999999.9 49572.25 152.3 81.9 999999.9 49607.25 178.5 103.2 999999.9 49642.25 145.4 999999.9 635.9 49677.25 124.4 999999.9 666.5 49712.25 164.0 999999.9 999999.9 49747.25 257.3 87.9 999999.9 49782.25 304.1 128.0 999999.9 49817.25 308.7 999999.9 999999.9 49852.25 446.6 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