44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 02 02 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 32813.13 -18.5 999999.9 0.0 32848.13 12.8 999999.9 0.0 32883.13 16.1 999999.9 0.0 32918.13 11.7 999999.9 0.0 32953.13 -0.5 999999.9 0.0 32988.13 7.2 999999.9 0.0 33023.13 -3.5 999999.9 0.0 33058.13 -9.5 17.6 0.0 33093.13 6.3 20.8 0.0 33128.13 11.7 999999.9 0.0 33163.13 29.3 999999.9 0.0 33198.13 18.1 999999.9 0.0 33233.13 33.7 999999.9 0.0 33268.13 41.4 23.6 0.0 33303.13 80.0 40.0 0.0 33338.13 154.9 999999.9 0.0 33373.13 146.8 999999.9 0.0 33408.13 125.5 999999.9 0.0 33443.13 166.8 999999.9 0.0 33478.13 167.5 999999.9 0.0 33513.13 217.8 88.1 0.0 33548.13 207.7 999999.9 0.0 33583.13 225.0 999999.9 0.0 33618.13 274.1 999999.9 0.0 33653.13 272.3 999999.9 0.0 33688.13 312.9 135.3 0.0 33723.13 365.3 179.4 0.0 33758.13 387.7 999999.9 0.0 33793.13 335.3 999999.9 0.0 33828.13 327.7 999999.9 0.0 33863.13 340.0 999999.9 0.0 33898.13 360.0 160.2 0.0 33933.13 457.3 196.4 0.0 33968.13 487.0 999999.9 0.0 34003.13 411.5 999999.9 0.0 34038.13 429.5 999999.9 0.0 34073.13 390.6 999999.9 0.0 34108.13 400.3 164.5 0.0 34143.13 392.2 129.2 0.0 34178.13 401.2 999999.9 0.0 34213.13 414.1 999999.9 0.0 34248.13 387.6 999999.9 0.0 34283.13 389.9 999999.9 0.0 34318.13 451.3 132.2 0.0 34353.13 598.9 187.7 0.0 34388.13 722.8 999999.9 0.0 34423.13 817.6 999999.9 0.0 34458.13 873.7 999999.9 0.0 34493.13 816.8 999999.9 0.0 34528.13 958.4 999999.9 0.0 34563.13 944.2 999999.9 0.0 34598.13 989.8 999999.9 0.0 34633.13 947.4 999999.9 0.0 34668.13 905.5 999999.9 0.0 34703.13 899.8 999999.9 0.0 34738.13 923.8 999999.9 0.0 34773.13 994.8 380.0 0.0 34808.13 970.4 405.8 0.0 34843.13 1000.4 999999.9 0.0 34878.13 987.7 999999.9 0.0 34913.13 958.7 999999.9 0.0 34948.13 990.8 999999.9 0.0 34983.13 1033.4 426.5 0.0 35018.13 1043.4 436.6 0.0 35053.13 1095.9 999999.9 0.0 35088.13 1114.7 999999.9 0.0 35123.13 1136.7 999999.9 0.0 35158.13 1110.6 999999.9 0.0 35193.13 1129.3 440.0 0.0 35228.13 1111.7 424.3 0.0 35263.13 1150.4 999999.9 0.0 35298.13 1135.9 999999.9 0.0 35333.13 1075.2 999999.9 0.0 35368.13 1113.6 999999.9 0.0 35403.13 1103.0 380.0 0.0 35438.13 1125.9 386.7 0.0 35473.13 1278.0 999999.9 0.0 35508.13 1196.3 999999.9 0.0 35543.13 1237.0 999999.9 0.0 35578.13 1161.3 999999.9 0.0 35613.13 1177.5 377.7 0.0 35648.13 1164.2 386.6 0.0 35683.13 1133.1 999999.9 0.0 35718.13 1130.5 999999.9 0.0 35753.13 1151.2 999999.9 0.0 35788.13 1156.5 999999.9 0.0 35823.13 1228.6 387.1 0.0 35858.13 1264.3 384.1 0.0 35893.13 1404.3 999999.9 0.0 35928.13 1290.0 999999.9 0.0 35963.13 1262.6 999999.9 0.0 35998.13 1283.6 999999.9 0.0 36033.13 1393.7 999999.9 0.0 36068.13 1362.7 999999.9 0.0 36103.13 1313.8 999999.9 0.0 36138.13 1325.8 999999.9 0.0 36173.13 1258.3 999999.9 0.0 36208.13 1265.9 999999.9 0.0 36243.13 1163.8 999999.9 0.0 36278.13 1119.5 343.9 0.0 36313.13 1188.5 375.7 0.0 36348.13 1156.2 999999.9 0.0 36383.13 1213.1 999999.9 0.0 36418.13 1223.4 999999.9 0.0 36453.13 1217.4 999999.9 0.0 36488.13 1219.8 377.1 0.0 36523.13 1160.7 360.6 0.0 36558.13 1281.3 999999.9 0.0 36593.13 1244.8 999999.9 0.0 36628.13 1217.3 999999.9 0.0 36663.13 1128.4 999999.9 0.0 36698.13 1135.4 346.3 0.0 36733.13 1089.3 325.4 0.0 36768.13 1109.2 999999.9 0.0 36803.13 1084.5 999999.9 0.0 36838.13 1111.4 999999.9 0.0 36873.13 1132.4 999999.9 0.0 36908.13 1117.1 328.3 0.0 36943.13 1147.6 314.1 0.0 36978.13 1173.2 999999.9 0.0 37013.13 1229.7 999999.9 0.0 37048.13 1223.9 999999.9 0.0 37083.13 1162.2 999999.9 0.0 37118.13 1212.1 373.8 0.0 37153.13 1185.8 377.0 0.0 37188.13 1163.0 999999.9 0.0 37223.13 1199.1 999999.9 0.0 37258.13 1204.0 999999.9 0.0 37293.13 1213.1 999999.9 0.0 37328.13 1256.7 386.1 0.0 37363.13 1239.2 383.5 0.0 37398.13 1320.7 999999.9 0.0 37433.13 1296.8 999999.9 0.0 37468.13 1292.2 999999.9 0.0 37503.13 1267.4 999999.9 0.0 37538.13 1370.6 999999.9 0.0 37573.13 1376.3 999999.9 0.0 37608.13 1360.7 999999.9 0.0 37643.13 1385.3 999999.9 0.0 37678.13 1324.3 999999.9 0.0 37713.13 1361.2 999999.9 0.0 37748.13 1357.4 999999.9 0.0 37783.13 1263.2 393.7 0.0 37818.13 1348.3 409.6 0.0 37853.13 1290.0 999999.9 0.0 37888.13 1330.6 999999.9 0.0 37923.13 1258.0 999999.9 0.0 37958.13 1325.9 999999.9 0.0 37993.13 1305.7 999999.9 0.0 38028.13 1290.8 402.3 0.0 38063.13 1388.6 999999.9 0.0 38098.13 1316.8 999999.9 0.0 38133.13 1388.1 999999.9 0.0 38168.13 1299.9 999999.9 0.0 38203.13 1254.1 382.2 0.0 38238.13 1227.7 366.2 0.0 38273.13 1288.9 999999.9 0.0 38308.13 1202.6 999999.9 0.0 38343.13 1154.2 999999.9 0.0 38378.13 1255.9 999999.9 0.0 38413.13 1188.7 999999.9 0.0 38448.13 1214.5 398.8 0.0 38483.13 1305.0 999999.9 0.0 38518.13 1281.9 999999.9 0.0 38553.13 1315.6 999999.9 0.0 38588.13 1323.5 999999.9 0.0 38623.13 1272.9 392.5 0.0 38658.13 1294.1 394.2 0.0 38693.13 1217.8 999999.9 0.0 38728.13 1282.6 999999.9 0.0 38763.13 1241.5 999999.9 0.0 38798.13 1269.2 999999.9 0.0 38833.13 1224.1 999999.9 0.0 38868.13 1217.7 398.7 0.0 38903.13 1334.3 999999.9 0.0 38938.13 1381.0 999999.9 0.0 38973.13 1351.0 999999.9 0.0 39008.13 1285.2 999999.9 0.0 39043.13 1434.6 999999.9 0.0 39078.13 1303.1 999999.9 0.0 39113.13 1330.8 999999.9 0.0 39148.13 1414.1 999999.9 0.0 39183.13 1330.7 999999.9 0.0 39218.13 1368.4 999999.9 0.0 39253.13 1287.1 999999.9 0.0 39288.13 1263.7 421.1 0.0 39323.13 1290.6 431.4 0.0 39358.13 1231.4 999999.9 0.0 39393.13 1188.4 999999.9 0.0 39428.13 1180.4 999999.9 0.0 39463.13 1242.0 999999.9 0.0 39498.13 1185.8 438.3 0.0 39533.13 1196.1 418.0 0.0 39568.13 1312.6 999999.9 0.0 39603.13 1275.5 999999.9 0.0 39638.13 1219.9 999999.9 0.0 39673.13 1266.0 999999.9 0.0 39708.13 1214.2 425.9 0.0 39743.13 1240.4 445.4 0.0 39778.13 1204.7 999999.9 0.0 39813.13 1192.6 999999.9 0.0 39848.13 1128.5 999999.9 0.0 39883.13 1237.2 999999.9 0.0 39918.13 1263.3 432.4 0.0 39953.13 1205.2 425.8 0.0 39988.13 1261.9 999999.9 0.0 40023.13 1228.3 999999.9 0.0 40058.13 1239.8 999999.9 0.0 40093.13 1206.2 999999.9 0.0 40128.13 1198.8 437.9 0.0 40163.13 1147.5 444.4 0.0 40198.13 1195.1 999999.9 0.0 40233.13 1149.8 999999.9 0.0 40268.13 1158.6 999999.9 0.0 40303.13 1178.2 999999.9 0.0 40338.13 1248.2 999999.9 0.0 40373.13 1194.2 468.7 0.0 40408.13 1242.3 999999.9 0.0 40443.13 1229.2 999999.9 0.0 40478.13 1198.2 999999.9 0.0 40513.13 1200.3 999999.9 0.0 40548.13 1288.9 999999.9 0.0 40583.13 1220.0 999999.9 0.0 40618.13 1253.9 999999.9 0.0 40653.13 1232.6 999999.9 0.0 40688.13 1147.0 999999.9 0.0 40723.13 1174.5 999999.9 0.0 40758.13 1135.6 999999.9 0.0 40793.13 1127.2 465.0 0.0 40828.13 1128.3 474.2 0.0 40863.13 1056.2 999999.9 0.0 40898.13 1074.5 999999.9 0.0 40933.13 1070.9 999999.9 0.0 40968.13 1069.0 999999.9 0.0 41003.13 1108.7 999999.9 0.0 41038.13 1062.8 506.9 0.0 41073.13 1176.5 999999.9 0.0 41108.13 1048.3 999999.9 0.0 41143.13 1118.2 999999.9 0.0 41178.13 1054.8 999999.9 0.0 41213.13 1033.0 534.7 0.0 41248.13 987.2 544.4 0.0 41283.13 1028.5 999999.9 0.0 41318.13 968.9 999999.9 0.0 41353.13 970.7 999999.9 0.0 41388.13 920.7 999999.9 0.0 41423.13 915.5 999999.9 0.0 41458.13 962.6 535.6 0.0 41493.13 1030.9 999999.9 0.0 41528.13 938.5 999999.9 0.0 41563.13 877.3 999999.9 0.0 41598.13 789.0 999999.9 0.0 41633.13 862.6 583.3 0.0 41668.13 866.7 579.3 0.0 41703.13 866.0 999999.9 0.0 41738.13 778.5 999999.9 0.0 41773.13 825.0 999999.9 0.0 41808.13 795.8 999999.9 0.0 41843.13 751.3 999999.9 0.0 41878.13 782.0 678.5 0.0 41913.13 770.8 999999.9 0.0 41948.13 747.0 999999.9 0.0 41983.13 720.3 999999.9 0.0 42018.13 664.3 999999.9 0.0 42053.13 710.8 999999.9 0.0 42088.13 671.8 999999.9 0.0 42123.13 667.0 999999.9 0.0 42158.13 691.1 999999.9 0.0 42193.13 606.3 999999.9 0.0 42228.13 593.7 999999.9 0.0 42263.13 571.5 999999.9 0.0 42298.13 552.2 710.6 0.0 42333.13 535.8 707.7 0.0 42368.13 526.7 999999.9 0.0 42403.13 525.9 999999.9 0.0 42438.13 491.0 999999.9 0.0 42473.13 488.4 999999.9 0.0 42508.13 457.6 703.8 0.0 42543.13 464.4 710.5 0.0 42578.13 525.5 999999.9 0.0 42613.13 464.8 999999.9 0.0 42648.13 470.5 999999.9 0.0 42683.13 496.1 999999.9 0.0 42718.13 499.3 737.7 0.0 42753.13 489.1 759.8 0.0 42788.13 498.3 999999.9 0.0 42823.13 491.2 999999.9 0.0 42858.13 470.5 999999.9 0.0 42893.13 430.5 999999.9 0.0 42928.13 454.4 999999.9 0.0 42963.13 428.8 794.7 0.0 42998.13 459.8 999999.9 0.0 43033.13 442.7 999999.9 0.0 43068.13 536.6 999999.9 0.0 43103.13 414.7 999999.9 0.0 43138.13 455.2 778.9 0.0 43173.13 385.9 791.5 0.0 43208.13 429.5 999999.9 0.0 43243.13 408.4 999999.9 0.0 43278.13 429.9 999999.9 0.0 43313.13 405.9 999999.9 0.0 43348.13 400.6 999999.9 0.0 43383.13 426.0 786.2 0.0 43418.13 417.7 999999.9 0.0 43453.13 385.3 999999.9 0.0 43488.13 407.1 999999.9 0.0 43523.13 453.1 999999.9 0.0 43558.13 432.7 999999.9 0.0 43593.13 408.9 999999.9 0.0 43628.13 447.6 999999.9 0.0 43663.13 443.0 999999.9 0.0 43698.13 407.9 999999.9 0.0 43733.13 425.4 999999.9 0.0 43768.13 363.4 999999.9 0.0 43803.13 345.1 779.9 0.0 43838.13 385.5 781.4 0.0 43873.13 417.3 999999.9 0.0 43908.13 381.4 999999.9 0.0 43943.13 369.0 999999.9 0.0 43978.13 365.3 999999.9 0.0 44013.13 380.8 999999.9 0.0 44048.13 386.9 811.8 0.0 44083.13 413.7 999999.9 0.0 44118.13 409.1 999999.9 0.0 44153.13 434.5 999999.9 0.0 44188.13 397.9 999999.9 0.0 44223.13 396.4 824.0 0.0 44258.13 367.4 815.4 0.0 44293.13 363.6 999999.9 0.0 44328.13 382.3 999999.9 0.0 44363.13 337.4 999999.9 0.0 44398.13 353.4 999999.9 0.0 44433.13 364.0 999999.9 0.0 44468.13 358.8 846.7 0.0 44503.13 354.1 999999.9 0.0 44538.13 347.2 999999.9 0.0 44573.13 354.4 999999.9 0.0 44608.13 345.3 999999.9 0.0 44643.13 313.5 843.1 0.0 44678.13 320.1 840.7 0.0 44713.13 330.6 999999.9 0.0 44748.13 348.4 999999.9 0.0 44783.13 321.6 999999.9 0.0 44818.13 298.1 999999.9 0.0 44853.13 305.8 999999.9 0.0 44888.13 294.4 820.3 0.0 44923.13 335.5 999999.9 0.0 44958.13 314.0 999999.9 0.0 44993.13 346.4 999999.9 0.0 45028.13 332.3 999999.9 0.0 45063.13 366.0 999999.9 0.0 45098.13 324.9 999999.9 0.0 45133.13 325.7 999999.9 0.0 45168.13 342.1 999999.9 0.0 45203.13 309.0 999999.9 0.0 45238.13 331.4 999999.9 0.0 45273.13 303.7 999999.9 0.0 45308.13 286.6 846.1 0.0 45343.13 293.9 853.6 0.0 45378.13 296.5 999999.9 0.0 45413.13 283.0 999999.9 0.0 45448.13 286.2 999999.9 0.0 45483.13 265.2 999999.9 0.0 45518.13 269.3 999999.9 0.0 45553.13 269.9 860.8 0.0 45588.13 273.3 999999.9 0.0 45623.13 297.4 999999.9 0.0 45658.13 300.7 999999.9 0.0 45693.13 282.8 999999.9 0.0 45728.13 293.8 805.7 0.0 45763.13 264.2 849.3 0.0 45798.13 275.3 999999.9 0.0 45833.13 262.8 999999.9 0.0 45868.13 249.2 999999.9 0.0 45903.13 267.4 999999.9 0.0 45938.13 263.5 999999.9 0.0 45973.13 290.4 816.6 0.0 46008.13 268.0 999999.9 0.0 46043.13 255.7 999999.9 0.0 46078.13 266.8 999999.9 0.0 46113.13 259.8 999999.9 0.0 46148.13 279.9 842.0 0.0 46183.13 268.1 860.8 0.0 46218.13 236.8 999999.9 0.0 46253.13 234.5 999999.9 0.0 46288.13 237.1 999999.9 0.0 46323.13 243.7 999999.9 0.0 46358.13 242.0 999999.9 0.0 46393.13 235.3 879.7 0.0 46428.13 250.8 999999.9 0.0 46463.13 242.5 999999.9 0.0 46498.13 226.5 999999.9 0.0 46533.13 260.3 999999.9 0.0 46568.13 254.5 999999.9 0.0 46603.13 239.9 999999.9 0.0 46638.13 248.8 999999.9 0.0 46673.13 264.6 999999.9 0.0 46708.13 229.5 999999.9 0.0 46743.13 249.1 999999.9 0.0 46778.13 258.5 999999.9 0.0 46813.13 211.5 865.4 0.0 46848.13 246.2 860.2 0.0 46883.13 241.7 999999.9 0.0 46918.13 213.5 999999.9 0.0 46953.13 230.7 999999.9 0.0 46988.13 208.8 999999.9 0.0 47023.13 232.5 999999.9 0.0 47058.13 222.4 911.8 0.0 47093.13 235.1 999999.9 0.0 47128.13 225.1 999999.9 0.0 47163.13 227.2 999999.9 0.0 47198.13 253.0 999999.9 0.0 47233.13 232.8 877.9 0.0 47268.13 197.7 905.4 0.0 47303.13 204.5 999999.9 0.0 47338.13 218.5 999999.9 0.0 47373.13 197.1 999999.9 0.0 47408.13 208.4 999999.9 0.0 47443.13 211.9 999999.9 0.0 47478.13 209.5 894.9 0.0 47513.13 214.4 999999.9 0.0 47548.13 233.8 999999.9 0.0 47583.13 220.5 999999.9 0.0 47618.13 223.8 999999.9 0.0 47653.13 194.8 907.5 0.0 47688.13 219.0 925.5 0.0 47723.13 204.7 999999.9 0.0 47758.13 199.6 999999.9 0.0 47793.13 199.6 999999.9 0.0 47828.13 204.8 999999.9 0.0 47863.13 201.9 999999.9 0.0 47898.13 191.0 896.8 0.0 47933.13 182.6 999999.9 0.0 47968.13 198.2 999999.9 0.0 48003.13 195.1 999999.9 0.0 48038.13 192.4 999999.9 0.0 48073.13 215.7 999999.9 0.0 48108.13 221.8 999999.9 0.0 48143.13 201.1 999999.9 0.0 48178.13 221.4 999999.9 0.0 48213.13 191.4 999999.9 0.0 48248.13 187.0 999999.9 0.0 48283.13 189.8 999999.9 0.0 48318.13 195.6 955.2 0.0 48353.13 187.8 934.1 0.0 48388.13 203.9 999999.9 0.0 48423.13 190.4 999999.9 0.0 48458.13 192.0 999999.9 0.0 48493.13 184.2 999999.9 0.0 48528.13 196.2 999999.9 0.0 48563.13 171.6 935.9 0.0 48598.13 195.5 999999.9 0.0 48633.13 181.7 999999.9 0.0 48668.13 202.3 999999.9 0.0 48703.13 169.6 999999.9 0.0 48738.13 164.9 878.8 0.0 48773.13 171.9 963.6 0.0 48808.13 188.6 999999.9 0.0 48843.13 179.7 999999.9 0.0 48878.13 184.2 999999.9 0.0 48913.13 173.9 999999.9 0.0 48948.13 167.0 999999.9 0.0 48983.13 165.8 903.5 0.0 49018.13 166.4 999999.9 0.0 49053.13 141.8 999999.9 0.0 49088.13 158.3 999999.9 0.0 49123.13 178.1 999999.9 0.0 49158.13 162.4 886.4 0.0 49193.13 174.0 869.9 0.0 49228.13 175.6 999999.9 0.0 49263.13 167.5 999999.9 0.0 49298.13 140.3 999999.9 0.0 49333.13 156.2 999999.9 0.0 49368.13 170.7 999999.9 0.0 49403.13 166.5 930.2 0.0 49438.13 163.3 999999.9 0.0 49473.13 179.8 999999.9 0.0 49508.13 157.2 999999.9 0.0 49543.13 165.7 999999.9 0.0 49578.13 155.1 999999.9 0.0 49613.13 155.5 999999.9 0.0 49648.13 149.1 999999.9 0.0 49683.13 164.4 999999.9 0.0 49718.13 181.0 999999.9 0.0 49753.13 160.2 999999.9 0.0 49788.13 176.3 999999.9 0.0 49823.13 173.7 956.7 0.0 49858.13 167.4 934.3 0.0 49893.13 168.1 999999.9 0.0 49928.13 158.3 999999.9 0.0 49963.13 144.9 999999.9 0.0 49998.13 159.8 999999.9 0.0 50033.13 156.3 999999.9 0.0 50068.13 145.8 907.1 0.0 50103.13 156.1 999999.9 0.0 50138.13 157.9 999999.9 0.0 50173.13 168.0 999999.9 0.0 50208.13 180.4 999999.9 0.0 50243.13 155.8 934.8 0.0 50278.13 133.8 909.7 0.0 50313.13 143.3 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